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Pressure effect on the competition between ferromagnetic and antiferromagnetic spin fluctuations in TmTe investigated by 125Te-NMR

Identifieur interne : 001608 ( Main/Exploration ); précédent : 001607; suivant : 001609

Pressure effect on the competition between ferromagnetic and antiferromagnetic spin fluctuations in TmTe investigated by 125Te-NMR

Auteurs : A. Yamamoto [Japon] ; S. Wada [Japon] ; T. Matsumura [Japon]

Source :

RBID : Pascal:07-0194304

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Abstract

To elucidate from a microscopic point of view the initial evolution of spin fluctuations in TmTe from the semiconducting state at ambient pressure with an antiferroquadrupole ordering (TQ = 1.8K) to the intermediate-valence metallic state at high pressures P≥2 GPa with a ferromagnetic (FM) ordering (Tc ≃ 14 K), we have carried out 125Te-NMR study at pressures P = 0 and 0.9 GPa. The spin-lattice relaxation rate measurements revealed a pronounced increase of the staggered susceptibility below T≃ 14 K, in addition to the Curie-Weiss-type increase of the uniform susceptibility. Below ∼T*, a wipe-out decrease of the NMR intensity and the finding of an unconventional NMR signal around ∼ 10 MHz that is insensitive to applied field lead to the conclusion that a field-induced short-range FM ordering caused by the competition of FM and antiferromagnetic fluctuations takes place. Pressure of 0.9 GPa hardly affects the anomalous NMR behaviors below T*, leading to speculate that the short-range FM ordering in the semiconducting state shares the origin with the long-range FM ordering at≃ 14K in the high-pressure metallic state.


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Le document en format XML

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<term>High pressure</term>
<term>Intermediate valence</term>
<term>Magnetic semiconductors</term>
<term>Nuclear magnetic resonance</term>
<term>Ordering</term>
<term>Pressure effects</term>
<term>Spin fluctuations</term>
<term>Spin-lattice relaxation</term>
<term>Thulium tellurides</term>
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<keywords scheme="Pascal" xml:lang="fr">
<term>Effet pression</term>
<term>Fluctuation spin</term>
<term>Résonance magnétique nucléaire</term>
<term>Relation ordre</term>
<term>Valence intermédiaire</term>
<term>Haute pression</term>
<term>Ferromagnétisme</term>
<term>Relaxation spin réseau</term>
<term>Loi Curie Weiss</term>
<term>Matériau ferromagnétique</term>
<term>Thulium tellurure</term>
<term>Semiconducteur magnétique</term>
<term>TmTe</term>
<term>7550P</term>
<term>7660</term>
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<div type="abstract" xml:lang="en">To elucidate from a microscopic point of view the initial evolution of spin fluctuations in TmTe from the semiconducting state at ambient pressure with an antiferroquadrupole ordering (T
<sub>Q</sub>
= 1.8K) to the intermediate-valence metallic state at high pressures P≥2 GPa with a ferromagnetic (FM) ordering (T
<sub>c</sub>
≃ 14 K), we have carried out
<sup>125</sup>
Te-NMR study at pressures P = 0 and 0.9 GPa. The spin-lattice relaxation rate measurements revealed a pronounced increase of the staggered susceptibility below T≃ 14 K, in addition to the Curie-Weiss-type increase of the uniform susceptibility. Below ∼T
<sup>*</sup>
, a wipe-out decrease of the NMR intensity and the finding of an unconventional NMR signal around ∼ 10 MHz that is insensitive to applied field lead to the conclusion that a field-induced short-range FM ordering caused by the competition of FM and antiferromagnetic fluctuations takes place. Pressure of 0.9 GPa hardly affects the anomalous NMR behaviors below
<sup></sup>
T
<sup>*</sup>
, leading to speculate that the short-range FM ordering in the semiconducting state shares the origin with the long-range FM ordering at≃ 14K in the high-pressure metallic state.</div>
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